Aarhus Universitets segl

No. 686 Danish emission inventories for road transport and other mobile sources

This report explains the emission inventories for road transport and other mobile sources, which are part of the annual Danish emission inventories reported to the UNFCCC (United Nations Framework Convention on Climate Change) and the UNECE LRTAP (United Nations Economic Commission for Europe Long Range Transboundary Pollution) conventions. The sub-sectors for other mobile sources are military, railways, navigation, fisheries, civil aviation and non-road machinery in agriculture, forestry, industry and household/gardening.

Table 0 . 1    Mobile sources and CRF codes

Mobile sources

CRF codes

Road transport

1A3b Transport-Road

Military

1A5 Other

Railways

1A3c Railways

Inland waterways

1A3d Transport-Navigation

National sea traffic

1A3d Transport-Navigation

National fishing

1A4c Agriculture/forestry/fisheries

International sea traffic

1A3d Transport-Navigation (international)

Dom. airport traffic 
(LTO < 1000 m)

1A3a Transport-Civil aviation

Int. airport traffic 
(LTO < 1000 m)

1A3a Transport-Civil aviation (international)

Dom. cruise traffic 
(> 1000 m)

1A3a Transport-Civil aviation

Int. cruise traffic 
(> 1000 m)

1A3a Transport-Civil aviation (international)

Agriculture

1A4c Agriculture/forestry/fisheries

Forestry

1A4c Agriculture/forestry/fisheries

Industry

1A2f Industry-Other

Household and gardening

1A4b Residential

 

 

 

The emissions of CO2, CH4, N2O, SO2, NOX, NMVOC, CO, NH3, particulate matter (PM), heavy metals, dioxins and PAH are shown in time-series as required by the UNFCCC and the UNECE LRTAP conventions, and grouped according to the UNFCCC Common Reporting Format (CRF) and UNECE National Format for Reporting (NFR) classification codes.

 

Methodologies

 

The emission calculations for road transport are made with an internal NERI model, with a structure similar to the European COPERT III (COmputer Programme to calculate the Emissions from Road Transport) methodology. The new emission factors from the updated COPERT IV version have been implemented in the NERI model. The emissions are calculated for operationally hot engines, during cold start and fuel evaporation. The model also includes the emission effect of catalyst wear. Input data for vehicle stock and mileage is obtained from the Danish Road Directorate, and is grouped according to average fuel consumption and emission behaviour. The emissions are estimated by combining vehicle and annual mileage numbers with hot emission factors, cold:hot ratios and evaporation factors.

 

For air traffic the 2001-2006 estimates are made on a city-pair level, using flight data from the Danish Civil Aviation Agency (CAA-DK) and landing/take off (LTO) and distance related emission factors from the EMEP/CORINAIR guidebook. For previous years the background data consist of LTO/aircraft type statistics from Copenhagen Airport and total LTO numbers from CAA-DK. With appropriate assumptions a consistent time-series of emissions is produced back to 1985 using also the findings from a Danish city-pair emission inventory in 1998.

 

For regional ferries, the fuel consumption and emissions are calculated as a product of number of round trips, sailing time per round trip, engine size, engine load factor and fuel consumption/emission factor. For small ferries and other national sea transport, the calculations are simply fuel based using the fuel consumption findings from a previous Danish research study in combination with average fuel related emission factors.

 

Non-road working machines and equipment, and recreational craft are grouped in the following sectors: Agriculture, Forestry, Industry, Household/Gardening and Inland Waterways. In general the emissions are calculated by combining information on the number of different machine types and their respective load factors, engine sizes, annual working hours and emission factors.

 

For military, railways and fisheries the emissions are calculated as the product of fuel use and emission factors.

 

Fuel sales data are obtained from the Danish energy statistics provided by the Danish Energy Authority (DEA). For road transport and aviation the emission results are adjusted in a fuel balance to ensure that all statistical fuel sold is accounted for in the calculations. For national sea transport, the fuel consumption of heavy oil and gas oil is calculated directly by NERI. Fuel adjustments are made in the fishery sector (gas oil) and stationary industry sources (heavy fuel oil) in order to maintain the grand national energy balance.

 

Emissions from road transport

 

Set in relation to the Danish national emission totals, the largest emission shares for road transport are noted for NOX, CO, CO2, NMVOC, TSP, PM2.5 and PM10. In 2006 the emission percentages were 36, 29, 23, 21, 12, 11 and 8, respectively. The emissions of NH3, N2O, CH4 and SO2 have marginal shares of 2.2, 1.9, 0.5 and 0.3 %, respectively.

 

From 1990 to 2006 the calculated emission changes for CO2 (and fuel use), CH4 and N2O are 36, -51 and 29 %. For NOX, NMVOC, CO and particulates (exhaust only: Size is below PM2.5), the 1985-2006 emission changes are -28, -71, -69, and -30 %.

 

The most significant emission changes from 1985 to 2006 occur for SO2 and NH3. For SO2 the emission drop is 99 % (due to reduced sulphur content in the diesel fuel), whereas the NH3 emissions increase by 3065 % (due to the introduction of catalyst cars).

Table 0 . 2    Emissions from road transport in 2006, changes from 1985 (19901) to 2006, and 2006 shares of national emission totals

CRF ID

SO2

NOX

NMVOC

CH4

CO

 

 

[tons]

[tons]

[tons]

[tons]

[tons]

 

Road (1A3b)

79

66993

23171

1290

171521

 

Total Road non-exhaust

 

 

 

 

 

 

Total Road

79

66993

23171

1290

171521

 

Total national, 2006

25048

185304

108182

262623

590599

 

Road- % of national, 2006

0.3

36

21

0.5

29

 

Road- % change 1985-2006

-99

-28

-71

-511

-69

 

CRF ID

CO2

N2O

NH3

TSP

PM10

PM2.5

 

[ktons]

[tons]

[tons]

[tons]

[tons]

[tons]

Road (1A3b)

12594

402

1951

3101

3101

3101

Total Road non-exhaust

 

 

 

2663

1726

937

Total Road

12594

402

1951

5764

4828

4039

Total national, 2006

55749

21026

89530

25048

38460

27726

Road- % of national, 2006

23

1.9

2.2

12

8.1

11

Road- % change 1985-2006

361

291

3065

-302

-302

-302

 

 

 

Road transport exhaust PM emissions almost solely come from diesel fuelled vehicles. The largest source is light duty trucks followed by heavy-duty vehicles and passenger cars in decreasing order. Since the mid-1990s the emissions from light and heavy duty vehicles have decreased significantly due to gradually stricter Euro emission standards. For diesel passenger cars, the environmental benefit of introducing new engines with lower particulate emissions since 1990 is more or less compensated by an increase in vehicle new sales in the later years.

 

The trend in non-exhaust PM follows the traffic growth in general, and in 2006 the TSP (total particulate matter), PM10 and PM2.5 shares were 46, 36 and 23 % of the respective road traffic totals. The non-exhaust PM is gaining more relative importance, in pace with the year by year reductions of exhaust PM.

 

Historically the emission totals of NOX and especially NMVOC and CO have been dominated by the contributions coming from gasoline passenger cars. However, the emissions from this vehicle type have been reduced since the introduction of catalyst cars in 1990. A negative side effect of this technology though is the increase in N2O and NH3 emissions. The NOX, NMVOC and CO emissions reductions are fortified by the introduction of new gradually stricter Euro emission standards for all other vehicle classes.

 

Emissions from other mobile sources

 

For other mobile sources the emissions of NOX, CO, NMVOC, TSP and PM2.5 have the largest shares of the national totals in 2006. The shares are 23, 21, 13, 10 and 9 %, respectively. The 2006 CO2, SO2 and PM10 emission shares are 7 %, whereas the emissions of N2O, NH3 and CH4 have marginal shares of 1 % or less in 2006.

 

From 1990 to 2006 the calculated emission changes for CO2 (and fuel use), CH4 and N2O are -10, 5 and -11 %. The emissions of SO2, particulates (all size fractions), NOX, NMVOC and CO have decreased by 88, 56, 14, 12 and 9 % from 1985 to 2006. For NH3 the emissions have increased by 8 % in the same time period.

Table 0 . 3     Emissions from other mobile sources in 2006, changes from 1985 (19903) to 2006, and 2006 shares of national emission totals

CRF ID

SO2

NOX

NMVOC

CH4

CO

 

 

[tons]

[tons]

[tons]

[tons]

[tons]

 

Industry-Other (1A2f)

30

10807

1583

44

7515

 

Civil Aviation (1A3a)

45

596

155

6

838

 

Railways (1A3c)

1

3542

230

9

626

 

Navigation (1A3d)

1089

7436

1195

32

7192

 

Residential (1A4b)

1

275

8037

233

87744

 

Ag./for./fish. (1A4c)

632

20199

2541

94

16976

 

Military (1A5)

26

619

56

6

391

 

Total other mobile

1824

43475

13796

425

121282

 

Total national, 2006

25048

185304

108182

262623

590599

 

Other mobile- % of national, 2006

7.3

23

13

0.2

21

 

Other mobile - % change 1985-2006

-88

-14

-12

53

-9

 

CRF ID

CO2

N2O

NH3

TSP

PM10

PM2.5

 

[ktons]

[tons]

[tons]

[tons]

[tons]

[tons]

Industry-Other (1A2f)

1021

43

2

991

991

991

Civil Aviation (1A3a)

141

8

0

3

3

3

Railways (1A3c)

227

6

1

120

120

120

Navigation (1A3d)

455

26

0

291

289

288

Residential (1A4b)

233

4

0

79

79

79

Ag./for./fish. (1A4c)

1599

77

3

1086

1084

1084

Military (1A5)

126

4

0

21

21

21

Total other mobile

3802

168

7

2590

2587

2585

Total national, 2006

55749

21026

89530

25048

38460

27726

Other mobile- % of national, 2006

6.8

0.8

0.0

10

6.7

9.3

Other mobile - % change 1985-2006

-103

-113

8

-56

-56

-56

 

 

 

The largest source of NOX and particulate emissions are agriculture/forestry/fisheries, followed by industry and navigation. For NMVOC and CO most of the emissions come from gasoline fuelled working machinery in the residential sector.

 

Heavy metals

 

For heavy metals the development in emissions follows the fuel use trends. The road transport shares for copper (Cu), zinc (Zn), chromium (Cr) and cadmium (Cd) are 71, 15, 15 and 6 % of national totals in 2006, and for other mobile sources the lead (Pb), Cu and nickel (Ni) shares are 21, 17 and 5 %. For the remaining components, the emission shares are less than 5 %.

 

The road transport emissions have increased by 36 % from 1990 to 2006. For Pb though there has been an almost 100 % emission decline, due to the phasing out of leaded gasoline fuels until 1994. For other mobile sources the emissions of Cd, Zn and Cu have emission decreases of 20 % or less in the same time period. The emissions of Pb, Ni, arsenic (Ar), selenium (Se), mercury (Hg) and Cr decrease even further. The respective emission declines are 79, 81, 68, 40, 26 and 23 %. For Ni, Se, Ar and Hg the emission decreases are due to a reduction in residual oil fuel use, and for Pb the reason for the emission drop is the contemporary phasing out of gasoline fuelled tractors and lead in gasoline fuel.

 

PAH’s

 

The PAH emission shares for road transport and other mobile sources are 5 % or less of the national total in 2006.

 

Uncertainties

 

For mobile sources in 2006 the CO2 emissions are determined with the highest accuracy, followed by the CH4, TSP, PM10, SO2, NMVOC, NOX, PM2.5, CO and N2O emissions with increasing levels of uncertainties. The uncertainties are 4, 34, 47, 48, 49, 49, 50, 50, 51 and 136 %, respectively. The uncertainties for the 1990-2006 emission trends are 4, 6, 8, 4, 10, 7, 7, 12 and 62 % for the emissions in the same consecutive order. For NH3, heavy metals and POPs the 2006 emissions have uncertainty levels of between 700 and 1000 %. In this case the emission trend uncertainties are significantly lower; still large fluctuations exist between the calculated values for the different emission components.

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